i think they're each other's favorite brother. they're together so often, and even though they try not to play favorites, it's a little obvious. they hang out a lot and have a lot of silly convos. ichimatsu has a few weird philosophies about the world, and jyushimatsu not only considers them, but adopts them, too! meanwhile, ichimatsu indulges in jyushimatsu's hobbies, like, uh... being walked on a leash.
i feel like the older/younger brother dynamic isn't huge with them because it doesn't need to be. they're brothers, and i think their relationship would be the same even if their ages switched, unlike some of the other brother dynamics.
notable moments/skits:
season 1 episode 5 — esp kitty
season 1 episode 17 — jyushimatsu and concepts
season 2 episode 17 — punishment
season 3 episode 19 — dogs